Moore was an authority on medieval and renaissance art and architecture and emeritus Professor of Art at Harvard University. From 1871 to 1879 he was an instructor in free hand drawing and water color at Harvard and for the next twelve years taught drawing and principles of design at the University. In 1891 he was appointed an assistant professor in Fine Arts, five years later was made professor of art, and in 1909 when he resigned his chair was designated Professor Emeritus. For some years he served as curator of the William Hayes Fogg Art Museum at Harvard and subsequently as director until the time of his retirement. He was the author of many books on art and architecture, among them “The Development and Character of Gothic Architecture”, “Examples for Elementary Practice in Delineation”, “Character of Renaissance Architecture”, and “Medieval Church Architecture of England.”